Ashikari, Yosuke and Tamaki, Takashi and Takahashi, Yusuke and Yao, Yiyue and Atobe, Mahito and Nagaki, Aiichiro (2022) Investigation of Parameter Control for Electrocatalytic Semihydrogenation in a Proton-Exchange Membrane Reactor Utilizing Bayesian Optimization. Frontiers in Chemical Engineering, 3. ISSN 2673-2718
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Abstract
Owing to its applicability in sustainable engineering, flow electrochemical synthesis in a proton-exchange membrane (PEM) reactor has attracted considerable attention. Because the reactions in PEM reactors are performed under electro-organic and flow-synthetic conditions, a higher number of reaction parameters exist compared to ordinary reactions. Thus, the optimization of such reactions requires significant amounts of energy, time, chemical and human resources. Herein, we show that the optimization of alkyne semihydrogenation in PEM reactors can be facilitated by means of Bayesian optimization, an applied mathematics strategy. Applying the optimized conditions, we also demonstrate the generation of a deuterated Z-alkene.
Item Type: | Article |
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Subjects: | Library Eprints > Chemical Science |
Depositing User: | Managing Editor |
Date Deposited: | 28 Jan 2023 06:20 |
Last Modified: | 29 Jul 2024 05:45 |
URI: | http://news.pacificarchive.com/id/eprint/1162 |